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Silver(II) fluoride

Silver(II) fluoride

Overview
Silver(II) fluoride is a chemical compound
Chemical compound
A chemical compound is a pure chemical substance consisting of two or more different chemical elements that can be separated into simpler substances by chemical reactions. Chemical compounds have a unique and defined chemical structure; they consist of a fixed ratio of atoms that are held together...

 with the formula
Chemical formula
A chemical formula or molecular formula is a way of expressing information about the atoms that constitute a particular chemical compound....

 AgF2. It is a rare example of a silver(II) compound. Silver is usually present in its +1 oxidation state
Oxidation state
In chemistry, the oxidation state is an indicator of the degree of oxidation of an atom in a chemical compound. The formal oxidation state is the hypothetical charge that an atom would have if all bonds to atoms of different elements were 100% ionic. Oxidation states are typically represented by...

. It is used as a fluorinating agent.

AgF2 can be synthesized by fluorinating Ag2O with elemental fluorine
Fluorine
Fluorine is the chemical element with atomic number 9, represented by the symbol F. Fluorine forms a single bond with itself in elemental form, resulting in the diatomic F2 molecule. F2 is a supremely reactive, poisonous, pale, yellowish brown gas. Elemental fluorine is the...

. Also, at 200 °C (473 K) elemental fluorine will react with AgF
Silver(I) fluoride
Silver fluoride , also known as argentous fluoride and silver monofluoride, is a compound of silver and fluorine. It is a ginger-coloured solid, melting point 435 °C, which blackens on exposure to moist air. Unlike other silver halides such as silver chloride it is soluble in water to the extent...

 or AgCl to produce AgF2.

As a strong fluorinating agent, AgF2 should be stored in Teflon or a passivated metal container.
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Encyclopedia
Silver(II) fluoride is a chemical compound
Chemical compound
A chemical compound is a pure chemical substance consisting of two or more different chemical elements that can be separated into simpler substances by chemical reactions. Chemical compounds have a unique and defined chemical structure; they consist of a fixed ratio of atoms that are held together...

 with the formula
Chemical formula
A chemical formula or molecular formula is a way of expressing information about the atoms that constitute a particular chemical compound....

 AgF2. It is a rare example of a silver(II) compound. Silver is usually present in its +1 oxidation state
Oxidation state
In chemistry, the oxidation state is an indicator of the degree of oxidation of an atom in a chemical compound. The formal oxidation state is the hypothetical charge that an atom would have if all bonds to atoms of different elements were 100% ionic. Oxidation states are typically represented by...

. It is used as a fluorinating agent.

Preparation


AgF2 can be synthesized by fluorinating Ag2O with elemental fluorine
Fluorine
Fluorine is the chemical element with atomic number 9, represented by the symbol F. Fluorine forms a single bond with itself in elemental form, resulting in the diatomic F2 molecule. F2 is a supremely reactive, poisonous, pale, yellowish brown gas. Elemental fluorine is the...

. Also, at 200 °C (473 K) elemental fluorine will react with AgF
Silver(I) fluoride
Silver fluoride , also known as argentous fluoride and silver monofluoride, is a compound of silver and fluorine. It is a ginger-coloured solid, melting point 435 °C, which blackens on exposure to moist air. Unlike other silver halides such as silver chloride it is soluble in water to the extent...

 or AgCl to produce AgF2.

As a strong fluorinating agent, AgF2 should be stored in Teflon or a passivated metal container. It is light sensitive.

AgF2 can be purchased from various suppliers, the demand being less than 100 kg/year. While laboratory experiments find use for AgF2, it is too expensive for large scale industry use. In 1993, AgF2 cost between 1000-1400 US dollars per kg.

Composition and structure


AgF2 is a white crystalline powder, but it is usually black/brown due to impurities. The F/Ag ratio for most samples is< 2, typically approaching 1.75 due to contamination with Ag
Silver
Silver is a chemical element with the chemical symbol Ag and atomic number 47. A soft, white, lustrous transition metal, it has the highest electrical conductivity of any element and the highest thermal conductivity of any metal...

 and oxides
Oxygen
Oxygen Oxygen Oxygen (acid, literally "sharp", from the taste of acids) and -γενής (-genēs) (producer, literally begetter) is the element with atomic number 8 and represented by the symbol O...

 and carbon
Carbon
Carbon is the chemical element with symbol C and atomic number 6. As a member of group 14 on the periodic table, it is nonmetallic and tetravalent—making four electrons available to form covalent chemical bonds...

.

For some time, it was doubted silver was actually in the 2+ oxidation state rather in some combination of states such as AgI[AgIIIF4], which would be similar to silver oxide. Neutron diffraction
Neutron diffraction
Neutron diffraction is a method for the determination of the atomic and/or magnetic structure of a material. It can be equally well applied to study crystalline solids , gasses, liquids or amorphous materials. Neutron diffraction is a form of elastic scattering where the neutrons exiting the...

 studies, however, confirmed its description as silver(II). The AgI[AgIIIF4] was found to be present at high temperatures, but it was unstable with respect to AgF2.

In the gas phase, AgF2 is believed to have D∞h symmetry
Symmetry group
The symmetry group of an object is the group of all isometries under which it is invariant with composition as the operation...

.

Approximately 14 kcal/mol
Mole (unit)
The mole is a unit of amount of substance: it is an SI base unit, and one of the few units used to measure this physical quantity. The name "mole" was coined in German by Wilhelm Ostwald in 1893, although the related concept of equivalent mass had been in use at least a century earlier...

 (59 kJ/mol) separate the ground  and first state
Excited state
Excitation is an elevation in energy level above an arbitrary baseline energy state. In physics there is a specific technical definition for energy level which is often associated with an atom being excited to an excited state....

s. The compound is paramagnetic, but it becomes ferromagnetic at temperatures below −110 °C (163 K).

Uses


AgF2 is a strong fluorinating and oxidation agent. Illustrative applications are listed below.
  • Fluoronation and preparation of organic perfluorocompounds

This type of reaction can occur in three different ways (here Z refers to any element or group attached to carbon, X is a halogen
Halogen
The halogens or halogen elements are a series of nonmetal elements from Group 17 IUPAC Style of the periodic table, comprising fluorine, ; chlorine, ; bromine, ; iodine, ; and astatine,...

):
1) CZ3H + 2 AgF2 → CZ3F +HF + 2 AgF
2) CZ3X + 2AgF2 → CZ3F +X2 + 2 AgF
3) Z2C=CZ2 + 2 AgF2 → Z2CFCFZ2 + 2 AgF

Similar transformations can also be effected using other high valence
Valence (chemistry)
In chemistry, valence, also known as valency or valency number, is a measure of the number of chemical bonds formed by the atoms of a given element...

 metallic fluorides such as CoF3
Cobalt(III) fluoride
Cobalt fluoride is the chemical compound with the formula CoF3. This highly reactive, hygroscopic brown solid is used to synthesize organofluorine compounds. CoF3 is a powerful fluorinating agent, the product being CoF2...

, MnF3, CeF4, and PbF4.
  • Fluorinations of aromatic compounds is readily achieved, but selective monofluorinations are more difficult:
C6H6 + 2 AgF2 → C6H5F + 2 AgF + HF

  • Oxidation of xenon
    Xenon
    Xenon is a chemical element represented by the symbol Xe. Its atomic number is 54. A colorless, heavy, odorless noble gas, xenon occurs in the Earth's atmosphere in trace amounts...

     . This reaction, which can be explosive, proceeds in anhydrous
    Anhydrous
    As a general term, a substance is said to be anhydrous if it contains no water. The way of achieving the anhydrous form differs from one substance to another.-Solvents:...

     HF solutions producing XeF2.

  • AgF2 oxidizes carbon monoxide
    Carbon monoxide
    Carbon monoxide is a colorless, odorless and tasteless gas, yet very toxic to humans. It consists of one carbon atom and one oxygen atom, connected by a covalent double bond and a dative covalent bond...

     to carbonyl fluoride
    Carbonyl fluoride
    Carbonyl fluoride is the chemical compound with the formula COF2. This gas, like its analogue phosgene, is highly toxic. The molecule is planar with C2v symmetry.-Safety:...

    .

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